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- W2887239391 abstract "Mesoporous [email protected] nanoplates, derived from zeolitic imidazolate framework-67 (ZIF-67) crystals, were facilely prepared via a silica-assisted strategy. Through introducing and removing colloidal silica during synthetic process, the [email protected] nanocomposites (CoOx@CS) exhibited mesopores characteristic and nanoplates. By comparison, the [email protected] nanocomposites (CoOx@C), obtained by a direct pyrolysis of ZIF-67, exhibited micropores characteristic and assembled microsphere. In catalytic decomposition of ammonia, it was found that the CoOx@CS nanocomposites showed excellent catalytic activity. Nearly 60% NH3 conversion was achieved at 500 °C with a space velocity of 6000 h−1, whereas only ~ 30% NH3 conversion was achieved under the same reaction conditions for CoOx@C nanocomposites. The enhanced activity should be attributed to mesoporous characteristic, nanoplates-like microstructure and basicity of carbon support. This study provides new insights into the development of controlling the structural orders of MOFs-derived carbon-based materials." @default.
- W2887239391 created "2018-08-22" @default.
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- W2887239391 date "2018-11-01" @default.
- W2887239391 modified "2023-10-08" @default.
- W2887239391 title "Silica-assisted mesoporous Co@Carbon nanoplates derived from ZIF-67 crystals and their enhanced catalytic activity" @default.
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- W2887239391 doi "https://doi.org/10.1016/j.jssc.2018.08.019" @default.
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