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• W2887301307 abstract "Abstract Two-dimensional (2D) magnetic materials with large spin polarization and high Curie temperature (Tc) are essential and indispensable for quantum computation, logic and memory operations, and spintronic devices at nanoscale. In this study, using the first-principles calculations based on the spin polarized density functional theory with the generalized gradient approximation (GGA) plus Hubbard-U corrections (GGA + U), we investigated the magnetic and electronic properties of 2D AlN sheets doped with different atoms of 3d transition metal (TM) elements. Our calculations demonstrate that these TM-doped 2D monolayer AlN sheets are magnetic semiconductors with integer magnetic moment. The magnetic moments of these doped systems originate mainly from the TM atoms, following the Hund's rule and crystal field theory. Furthermore, we find that the magnetic coupling in the Mn- and Ni-doped 2D AlN sheets is ferromagnetic, while the magnetic coupling in the other TM-doped 2D AlN sheets is anti-ferromagnetic. For the ferromagnetic and semiconducting TM-doped monolayer AlN sheets, the calculated Curie temperatures are above 400 K, exceeding that (155 K) of the most-studied dilute magnetic GaMnAs material. Our studies suggest that the Mn- and Ni-doped 2D monolayer AlN sheets would show very promising applications in the spintronic device at nanoscale." @default.
• W2887301307 created "2018-08-22" @default.
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• W2887301307 date "2018-10-01" @default.
• W2887301307 modified "2023-09-24" @default.
• W2887301307 title "First-principles prediction of ferromagnetism in transition-metal doped monolayer AlN" @default.
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• W2887301307 doi "https://doi.org/10.1016/j.spmi.2018.08.009" @default.
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