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• W2887757488 abstract "A formal total synthesis of the antitumor marine natural product (rac)-renieramycin T, which possesses a characteristic ecteinascidin-type A ring in the renieramycin-saframycin core skeleton, was elaborated. The key steps in the synthesis of (rac)-renieramycin T are a modified Pictet-Spengler cyclization of dialkylated oxomalonate derivatives and decarboxylation via a monocarboxylic acid derivative followed by stereocontrolled protonation of the enol intermediate. A key intermediate in our previous synthesis of renieramycin T was used, and the formal synthesis was accomplished in 21 steps from a known piperazine-2,5-dione derivative." @default.
• W2887757488 created "2018-08-22" @default.
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• W2887757488 date "2018-08-07" @default.
• W2887757488 modified "2023-10-15" @default.
• W2887757488 title "Construction of the Pentacyclic Core and Formal Total Synthesis of (<i>rac</i>)‐Renieramycin T" @default.
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• W2887757488 doi "https://doi.org/10.1002/open.201800112" @default.
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