FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W2887863345> ?p ?o ?g. }

• W2887863345 endingPage "8455" @default.
• W2887863345 startingPage "8447" @default.
• W2887863345 abstract "The excitation of localized surface plasmon resonances in Au and Ag colloids can be used to drive the synthesis of complex nanostructures, such as anisotropic prisms, bipyramids, and core@shell nanoparticles. Yet, after two decades of research, it is challenging to paint a complete picture of the mechanisms driving such light-induced chemical transformations. In particular, whereas the injection of hot charge carriers from the metal nanoparticles is usually proposed as the dominant mechanism, the contribution of plasmon-induced heating can often not be neglected. Here, we tackle this uncertainty and quantify the contribution of different activation mechanisms using a temperature-sensitive synthesis of Au@Ag core@shell nanoparticles. We compare the rate of Ag shell growth in the dark at different temperatures with the one under plasmon excitation with varying laser intensities. Our controlled illumination geometry, coupled to numerical modeling of light propagation and heat diffusion in the reaction volume, allows us to quantify both localized and collective heating effects and determine their contribution to the total growth rate of the nanoparticles. We find that nonthermal effects can be dominant, and their relative contribution depends on the fraction of nanoparticle suspension under irradiation. Understanding the mechanism of plasmon-activated chemistry at the surface of metal nanoparticles is of paramount importance for a wide range of applications, from the rational design of novel light-assisted nanoparticle syntheses to the development of plasmonic nanostructures for catalytic and therapeutic purposes." @default.
• W2887863345 created "2018-08-22" @default.
• W2887863345 creator A5005309801 @default.
• W2887863345 creator A5010833315 @default.
• W2887863345 creator A5043024418 @default.
• W2887863345 creator A5068754422 @default.
• W2887863345 creator A5080208003 @default.
• W2887863345 date "2018-08-02" @default.
• W2887863345 modified "2023-10-14" @default.
• W2887863345 title "Quantifying Photothermal and Hot Charge Carrier Effects in Plasmon-Driven Nanoparticle Syntheses" @default.
• W2887863345 cites W1521131431 @default.
• W2887863345 cites W1972560232 @default.
• W2887863345 cites W2010467127 @default.
• W2887863345 cites W2013492930 @default.
• W2887863345 cites W2014840512 @default.
• W2887863345 cites W2025864704 @default.
• W2887863345 cites W2037816827 @default.
• W2887863345 cites W2045276693 @default.
• W2887863345 cites W2073409644 @default.
• W2887863345 cites W2074587918 @default.
• W2887863345 cites W2075765693 @default.
• W2887863345 cites W2082994362 @default.
• W2887863345 cites W2083926174 @default.
• W2887863345 cites W2084279813 @default.
• W2887863345 cites W2088525842 @default.
• W2887863345 cites W2089210645 @default.
• W2887863345 cites W2092539730 @default.
• W2887863345 cites W2092648672 @default.
• W2887863345 cites W2108069322 @default.
• W2887863345 cites W2117037705 @default.
• W2887863345 cites W2119767565 @default.
• W2887863345 cites W2126703845 @default.
• W2887863345 cites W2128544853 @default.
• W2887863345 cites W2132441274 @default.
• W2887863345 cites W2132667015 @default.
• W2887863345 cites W2137756244 @default.
• W2887863345 cites W2156750191 @default.
• W2887863345 cites W2161989523 @default.
• W2887863345 cites W2165075822 @default.
• W2887863345 cites W2171581030 @default.
• W2887863345 cites W2194481299 @default.
• W2887863345 cites W2229224778 @default.
• W2887863345 cites W2277286098 @default.
• W2887863345 cites W2312248536 @default.
• W2887863345 cites W2314027892 @default.
• W2887863345 cites W2326708413 @default.
• W2887863345 cites W2342652847 @default.
• W2887863345 cites W2413685977 @default.
• W2887863345 cites W2474650414 @default.
• W2887863345 cites W2644600533 @default.
• W2887863345 cites W2738514020 @default.
• W2887863345 cites W2788642740 @default.
• W2887863345 cites W3007580766 @default.
• W2887863345 cites W4233799981 @default.
• W2887863345 doi "https://doi.org/10.1021/acsnano.8b03929" @default.
• W2887863345 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30071160" @default.
• W2887863345 hasPublicationYear "2018" @default.
• W2887863345 type Work @default.
• W2887863345 sameAs 2887863345 @default.
• W2887863345 citedByCount "65" @default.
• W2887863345 countsByYear W28878633452019 @default.
• W2887863345 countsByYear W28878633452020 @default.
• W2887863345 countsByYear W28878633452021 @default.
• W2887863345 countsByYear W28878633452022 @default.
• W2887863345 countsByYear W28878633452023 @default.
• W2887863345 crossrefType "journal-article" @default.
• W2887863345 hasAuthorship W2887863345A5005309801 @default.
• W2887863345 hasAuthorship W2887863345A5010833315 @default.
• W2887863345 hasAuthorship W2887863345A5043024418 @default.
• W2887863345 hasAuthorship W2887863345A5068754422 @default.
• W2887863345 hasAuthorship W2887863345A5080208003 @default.
• W2887863345 hasBestOaLocation W28878633452 @default.
• W2887863345 hasConcept C10165471 @default.
• W2887863345 hasConcept C104232198 @default.
• W2887863345 hasConcept C106847996 @default.
• W2887863345 hasConcept C110879396 @default.
• W2887863345 hasConcept C136676167 @default.
• W2887863345 hasConcept C147789679 @default.
• W2887863345 hasConcept C155672457 @default.
• W2887863345 hasConcept C159467904 @default.
• W2887863345 hasConcept C171250308 @default.
• W2887863345 hasConcept C182606246 @default.
• W2887863345 hasConcept C185592680 @default.
• W2887863345 hasConcept C186187911 @default.
• W2887863345 hasConcept C192562407 @default.
• W2887863345 hasConcept C2780358262 @default.
• W2887863345 hasConcept C49040817 @default.
• W2887863345 hasConcept C85255121 @default.
• W2887863345 hasConceptScore W2887863345C10165471 @default.
• W2887863345 hasConceptScore W2887863345C104232198 @default.
• W2887863345 hasConceptScore W2887863345C106847996 @default.
• W2887863345 hasConceptScore W2887863345C110879396 @default.
• W2887863345 hasConceptScore W2887863345C136676167 @default.
• W2887863345 hasConceptScore W2887863345C147789679 @default.
• W2887863345 hasConceptScore W2887863345C155672457 @default.
• W2887863345 hasConceptScore W2887863345C159467904 @default.
• W2887863345 hasConceptScore W2887863345C171250308 @default.
• W2887863345 hasConceptScore W2887863345C182606246 @default.

• next