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• W2888584866 abstract "Resonance energy transfer (RET) is a complex phenomenon where energy is transferred between two nonequivalent molecules. In the Förster picture, that applies to the weak coupling regime, RET occurs from the energy donor molecule in the relaxed excited state toward the acceptor, in an energy-conserving process. However, energy dissipation is crucial for a more general picture of RET that also applies to the strong coupling regime. Here we present a dynamical, nonadiabatic model for RET also accounting for energy relaxation. We exploit the essential state formalism to set up a model for the RET pair that yields an accurate picture of the relevant physics, accounting for just a few electronic states and a single coupled vibrational coordinate per molecule. Molecular vibrations are treated in a nonadiabatic approach, and energy dissipation is dealt within the Redfield formalism. The approach is first validated on an isolated dye, demonstrating that a very simple relaxation model, defined in terms of a single relaxation parameter, properly describes the different regimes of energy dissipation expected for a molecule, with a fast (fs time window) internal conversion to the lowest excited state and a slow relaxation toward the ground state (ns time window). The same approach is then applied to follow the real time dynamics of a RET pair. In line with the Förster model, in the weak coupling regime the internal conversion of the donor molecule is completed before energy transfer takes place. Our approach also applies to the strong coupling regime, where we observe ultrafast energy transfer occurring well before the internal relaxation of the energy donor is completed." @default.
• W2888584866 created "2018-08-31" @default.
• W2888584866 creator A5038650505 @default.
• W2888584866 creator A5091344365 @default.
• W2888584866 date "2018-08-24" @default.
• W2888584866 modified "2023-09-24" @default.
• W2888584866 title "Intermolecular Energy Transfer in Real Time" @default.
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• W2888584866 cites W1977289260 @default.
• W2888584866 cites W1977964292 @default.
• W2888584866 cites W1981517702 @default.
• W2888584866 cites W1983149290 @default.
• W2888584866 cites W1984918795 @default.
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• W2888584866 cites W2004830905 @default.
• W2888584866 cites W2005763224 @default.
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• W2888584866 doi "https://doi.org/10.1021/acs.jctc.8b00540" @default.
• W2888584866 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30141921" @default.
• W2888584866 hasPublicationYear "2018" @default.
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