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- W2888756095 abstract "Abstract Transformation of greenhouse gas CO 2 and renewable H 2 into fuels and commodity chemicals is recognized as a promising route to store fluctuating renewable energy. Although several C 1 chemicals, olefins, and gasoline have been successfully synthesized by CO 2 hydrogenation, selective conversion of CO 2 and H 2 into aromatics is still challenging due to the high unsaturation degree and complex structures of aromatics. Here we report a composite catalyst of ZnAlO x and H-ZSM-5 which yields high aromatics selectivity (73.9%) with extremely low CH 4 selectivity (0.4%) among the carbon products without CO. Methanol and dimethyl ether, which are synthesized by hydrogenation of formate species formed on ZnAlO x surface, are transmitted to H-ZSM-5 and subsequently converted into olefins and finally aromatics. Furthermore, 58.1% p -xylene in xylenes is achieved over the composite catalyst containing Si-H-ZSM-5. ZnAlO x &H-ZSM-5 suggests a promising application in manufacturing aromatics from CO 2 and H 2 ." @default.
- W2888756095 created "2018-08-31" @default.
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- W2888756095 date "2018-08-27" @default.
- W2888756095 modified "2023-10-18" @default.
- W2888756095 title "Selective conversion of CO2 and H2 into aromatics" @default.
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- W2888756095 doi "https://doi.org/10.1038/s41467-018-05880-4" @default.
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