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• W2889572425 abstract "Schiff-condensation reactions carried out between 1,6-diaminopyrene (DAP) and the tritopical 1,3,5 benzenetricarbaldehyde (BTCA) or 2,4,6-triformylphloroglucinol (TP) ligands give rise to the formation of two-dimensional imine-based covalent-organic frameworks (COFs), named IMDEA-COF-1 and -2, respectively. These materials show dramatic layer-packing-driven fluorescence in solid state arising from the three-dimensional arrangement of the pyrene units among layers. Layer stacking within these 2D-COF materials to give either eclipsed or staggered conformations can be controlled, at an atomic level through chemical design of the building blocks used in their synthesis. Theoretical calculations have been used to rationalize the different preferential packing between both COFs. IMDEA-COF-1 shows green emission with absolute photoluminescence quantum yield of 3.5% in solid state. This material represents the first example of imine-linked 2D-COF showing emission in solid state." @default.
• W2889572425 created "2018-09-27" @default.
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• W2889572425 date "2018-09-14" @default.
• W2889572425 modified "2023-10-16" @default.
• W2889572425 title "Layer-Stacking-Driven Fluorescence in a Two-Dimensional Imine-Linked Covalent Organic Framework" @default.
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• W2889572425 doi "https://doi.org/10.1021/jacs.8b07450" @default.
• W2889572425 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30216717" @default.
• W2889572425 hasPublicationYear "2018" @default.
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