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• W2889650126 abstract "The salt removal capacity (SRC) of the carbon electrodes in membrane capacitive deionization (MCDI) is limited by the applied potential (<1.6 V). Thus, enhancement of the SRC is essential before applying MCDI to seawater desalination. This study aims at developing a novel MCDI system for seawater desalination by applying over-potential (OP) to enhance ion-adsorption capacity and kinetics, and by reversing the polarity (RP) of electrodes to improve ion-desorption kinetics (hereafter named OP-MCDI-RP) for seawater desalination. At 2.4 V, the OP-MCDI system with mesoporous carbon demonstrated a SRC value of 64.7 mg g−1 when desalting 0.5 M NaCl solution, while the OP-CDI system could only remove 8.2 mg g−1 under identical conditions. Similarly, an OP-MCDI cell using carbon aerogel demonstrated a greater SRC value of 43.4 mg g−1 in comparison with 12.5 mg g−1 achieved in OP-CDI. These results indicate that the OP-MCDI system can directly desalt high salinity water regardless of the electrode material. In contrast to the OP-MCDI system, the OP-MCDI-RP system yields a higher regeneration efficiency by applying a reversed low-voltage. It is shown that, under appropriate operating conditions, the OP-MCDI-RP system reduced the electrical conductivity of a seawater sample of 37 practical salinity units by 99.9%, suggesting that the OP-MCDI-RP system can be employed for seawater desalination. Due to the dramatic increase in energy demand and insufficient long-term stability caused by high potential and high salt concentration, however, the OP-MCDI-RP process should be further investigated for potential practical applications." @default.
• W2889650126 created "2018-09-27" @default.
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• W2889650126 date "2019-02-01" @default.
• W2889650126 modified "2023-10-14" @default.
• W2889650126 title "Seawater desalination by over-potential membrane capacitive deionization: Opportunities and hurdles" @default.
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• W2889650126 doi "https://doi.org/10.1016/j.cej.2018.09.121" @default.
• W2889650126 hasPublicationYear "2019" @default.
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