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• W2889779913 abstract "Rational design of oxygen reduction reaction (ORR) electrocatalysts based on earth-abundant elements is critical important towards sustainable energy applications. Among various reported ORR electrocatalysts, transition metal-nitrogen doped carbon (TM-N/C) materials such as Fe-Nx/C and Co-Nx/C exhibit excellent catalytic activity. Nevertheless, comprehensive understanding of these TM-N/C electrocatalytic systems is still lacking, which demands extension of investigation to other TM-N/C systems (Cu, and Mn, etc.). Herein, we developed a Cu promoted nitrogen-doped carbon (Cu-N/C) via high temperature pyrolysis of Cu-adsorbed zeolite imidazole frameworks (Cu@ZIF-8). The Cu-N/C electrocatalyst exhibited satisfactory ORR activity with half-wave potential of 0.813 V in 0.1 M KOH electrolyte. Moreover, it also showed excellent methanol tolerance and long-term stability. The enhanced ORR electrocatalytic performance is attributed to the strong synergetic effect between Cu(II)-N ligands and Cu0 NPs, sufficient active sites, and fast mass transfer." @default.
• W2889779913 created "2018-09-27" @default.
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• W2889779913 date "2019-01-01" @default.
• W2889779913 modified "2023-10-16" @default.
• W2889779913 title "Copper-promoted nitrogen-doped carbon derived from zeolitic imidazole frameworks for oxygen reduction reaction" @default.
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• W2889779913 doi "https://doi.org/10.1016/j.apsusc.2018.09.102" @default.
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