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• W2890101239 abstract "A regio- and stereoselective silver-catalyzed formal carbene insertion into 1,3-dicarbonyls has been developed, using N-nosylhydrazones as diazo surrogates. Two new C−C bonds are constructed at the carbenic carbon center through the selective cleavage of the C−C(=O) σ-bond of acyclic 1,3-dicarbonyls, enabling the preparation of various synthetically useful polysubstituted γ-diketones, γ-ketoesters, and γ-ketoamides in high yields. The in situ formation of a donor-acceptor cyclopropane, via reaction of the enolate of the 1,3-dicarbonyl with an electrophilic silver carbenoid, is proposed as a key process in the catalytic cycle." @default.
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• W2890101239 date "2018-10-01" @default.
• W2890101239 modified "2023-10-14" @default.
• W2890101239 title "Silver-Catalyzed Regio- and Stereoselective Formal Carbene Insertion into Unstrained C−C σ-Bonds of 1,3-Dicarbonyls" @default.
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• W2890101239 doi "https://doi.org/10.1016/j.isci.2018.09.006" @default.
• W2890101239 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/6170519" @default.
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