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- W2890108228 abstract "Combustion ChemistryThe chemical origin of soot is a persistent puzzle. It is clear that small hydrocarbon fragments formed in flames must aggregate into larger particles, but the initial driving force for aggregation remains a mystery. Johansson et al. combined theory and mass spectrometry to suggest a solution based on resonance-stabilized radicals (see the Perspective by Thomson and Mitra). Aromatics such as cyclopentadiene have a characteristically weak C–H bond because their cleavage produces radicals with extended spans of π-electron conjugation. Clusters thus build up through successive coupling reactions that extend conjugation in stabilized radicals of larger and larger size.Science , this issue p. [997][1]; see also p. [978][2] [1]: /lookup/doi/10.1126/science.aat3417 [2]: /lookup/doi/10.1126/science.aau5941" @default.
- W2890108228 created "2018-09-27" @default.
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- W2890108228 date "2018-09-06" @default.
- W2890108228 modified "2023-09-25" @default.
- W2890108228 title "A radical route to soot" @default.
- W2890108228 doi "https://doi.org/10.1126/science.361.6406.987-r" @default.
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