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- W2890112158 abstract "Herein, we broaden the application scope of (cyclopentadienone)iron complexes 1 in C=N bond reduction. The catalytic scope of pre‐catalyst 1b , which is more active than the “Knölker complex” ( 1a ) and other members of its family, has been expanded to the catalytic transfer hydrogenation (CTH) of a wider range of aldimines and ketimines, either pre‐isolated or generated in situ. The kinetics of 1b ‐promoted CTH of ketimine S1 were assessed, showing a pseudo‐first order profile, with TOF = 6.07 h –1 at 50 % conversion. Moreover, the chiral complex 1c and its analog 1d were employed in the enantioselective reduction of ketimines and reductive amination of ketones, giving fair to good yields and moderate enantioselectivity." @default.
- W2890112158 created "2018-09-27" @default.
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- W2890112158 date "2018-10-12" @default.
- W2890112158 modified "2023-10-12" @default.
- W2890112158 title "Improving C=N Bond Reductions with (Cyclopentadienone)iron Complexes: Scope and Limitations" @default.
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- W2890112158 doi "https://doi.org/10.1002/ejoc.201801348" @default.
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