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- W2890118317 abstract "Abstract A novel organocatalytic approach to γ,γ‐disubstituted butenolides is described. It is based on a fully site‐selective functionalization of 5‐alkylidenefuran‐2(5 H )‐ones via trienamine‐mediated [4+2]‐cycloaddition with α,β,γ,δ‐diunsaturated aldehydes. The developed methodology proceeds with excellent stereocontrol and constitutes a unique example of trienamine chemistry with vinylogous dienophiles. Importantly, the reaction has very broad scope and allows for the introduction of substituents also in the α‐ or the β‐position of the butenolide ring. Usefulness of the products obtained has been confirmed in the intramolecular Stetter reaction leading to polycyclic product." @default.
- W2890118317 created "2018-09-27" @default.
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- W2890118317 date "2018-10-19" @default.
- W2890118317 modified "2023-10-12" @default.
- W2890118317 title "Synthesis of γ,γ-Disubstituted Butenolides through a Doubly Vinylogous Organocatalytic Cycloaddition" @default.
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- W2890118317 doi "https://doi.org/10.1002/chem.201804650" @default.
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