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• W2890157030 abstract "We report herein HMF (5-hydroxymethylfurfural) and furfural oxidation to 2,5-furandicarboxylic (FDCA) and furoic acids, respectively, in water, under base-free conditions and using supported gold nanoparticles. Prepared catalysts showed high catalytic activity under environmentally friendly conditions. Especially, the use of base-free conditions enables getting rid of the most usually needed neutralization step generating salts that must be further handled/eliminated. We showed that the conversion and the selectivity to desired products depend on the basicity of the support. To this respect, the Au/MgO catalyst was the most active sample (100% and 90% yields to furoic acid and 2,5-furandicarboxylic acid, respectively), although a partial leaching of Mg was observed (89 ppm). Novel Au/MgF2-MgO catalysts were also very active (97% yield of furoic acid) with a final pH of 7.5. High yields of acid were also obtained (78%) with an acid final pH of 3.8, actually enabling the isolation of products under their acid form directly from the reaction medium without a neutralization step." @default.
• W2890157030 created "2018-09-27" @default.
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• W2890157030 date "2018-09-13" @default.
• W2890157030 modified "2023-10-14" @default.
• W2890157030 title "Influence of Support Basic Sites in Green Oxidation of Biobased Substrates Using Au-Promoted Catalysts" @default.
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• W2890157030 doi "https://doi.org/10.1021/acssuschemeng.8b03330" @default.
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