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• W2890178686 abstract "Self-discharge performance is one of the key indexes of nickel-metal hydride batteries. In this work, single-phase Ce2Ni7-type La–Nd–Mg–Ni-based alloy with great application potential in long-term storage Ni/MH batteries are prepared by step-wise annealing. The as-cast alloy contains CaCu5-, Gd2Co7- and Ce5Co19-type phases. After annealed at 1248 K, CaCu5- and Ce5Co19-type phases disappear and a single-phase Gd2Co7-type structure is obtained. With the temperature increase, Gd2Co7-type structure begins to transform into Ce2Ni7-type structure. As annealed at 1323 K, the alloy shows a Ce2Ni7-type single-phase structure. The C60 (discharge capacity at 60 mA g−1) of Ce2Ni7-type electrode reaches 405 mAh g−1, and the C1900 is even high to 210 mAh g−1. The Ce2Ni7-type electrode also shows superior self-discharge properties and the charge retention rate for 1 d (CRT1d) is 96.5%. Moreover after 150 cycles, the CRT1d is even high to 97.7% and CRT7d is 81.5%. While those of the as-cast electrodes are only 79% and 36%, respectively. Electrochemical pressure-composition isotherms show that Ce2Ni7-type electrode has relatively lower hydrogen desorption plateau pressure, indicating more stable hydride and less reversible self-discharge. After 150 cycles, the plateau pressure gets even lower. Moreover Ce2Ni7-type electrode possesses smaller corrosion current density, indicating minor oxidation/corrosion degree." @default.
• W2890178686 created "2018-09-27" @default.
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• W2890178686 date "2018-01-01" @default.
• W2890178686 modified "2023-10-15" @default.
• W2890178686 title "Self-Discharge Characteristic of La0.60Nd0.15Mg0.25Ni3.50 Alloy with Single-Phase Ce2Ni7-Type Super-Stacking Structure" @default.
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• W2890178686 doi "https://doi.org/10.1149/2.1241811jes" @default.
• W2890178686 hasPublicationYear "2018" @default.
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