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• W2890180722 abstract "In the present work, a rapid and novel route to prepare a diblock copolymer consisting of styrene and vinyl acetate (VAC) units was performed by successive photoinduced charge-transfer polymerization (CTP) under UV irradiation, and then a series of objective products PS m -b-PVA n bearing different ratios of PS and PVA was obtained by the hydrolysis of PS m -b-PVAC n with sodium ethoxide as the catalyst. Additionally, the influences of the reaction time, concentration of monomer and photoinitiator and kinetics of copolymerization were investigated. Good linear relationships of ln([St] 0 /[St]) and ln([VAc] 0 /[VAc]) with the polymerization time indicated a first-order control/‘living’ process. The copolymers were characterized in detail by means of Fourier transform infrared (IR) spectrometry, 1 H NMR and gel permeation chromatography (GPC). Furthermore, the miscibility of the originally incompatible blend system was improved quite significantly, so a full atomistic molecular dynamics simulation was applied to discuss the binary and ternary systems through the Flory-Huggins parameters, enthalpy of mixing and T g ." @default.
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• W2890180722 date "2015-07-01" @default.
• W2890180722 modified "2023-09-26" @default.
• W2890180722 title "Synthesis of Poly (Styrene-Block-Vinyl Alcohol) by Successive Photo-Induced Charge Transfer Polymerization and Molecular Dynamics Simulation of Its Compatibility for the Blend System" @default.
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• W2890180722 doi "https://doi.org/10.1177/096739111502300607" @default.
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