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- W2890192850 abstract "Abstract The ability to modulate nanoparticle (NP) assemblies with atomic precision is still lacking, which hinders us from creating hierarchical NP organizations with desired properties. In this work, a hierarchical fibrous (1D to 3D) assembly of Au NPs (21-gold atom, Au 21 ) is realized and further modulated with atomic precision via site-specific tailoring of the surface hook (composed of four phenyl-containing ligands with a counteranion). Interestingly, tailoring of the associated counterion significantly changes the electrical transport properties of the NP-assembled solids by two orders of magnitude due to the altered configuration of the interacting π–π pairs of the surface hooks. Overall, our success in atomic-level modulation of the hierarchical NP assembly directly evidences how the NP ligands and associated counterions can function to guide the 1D, 2D, and 3D hierarchical self-assembly of NPs in a delicate manner. This work expands nanochemists’ skills in rationally programming the hierarchical NP assemblies with controllable structures and properties." @default.
- W2890192850 created "2018-09-27" @default.
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- W2890192850 date "2018-09-24" @default.
- W2890192850 modified "2023-10-17" @default.
- W2890192850 title "Modulating the hierarchical fibrous assembly of Au nanoparticles with atomic precision" @default.
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- W2890192850 doi "https://doi.org/10.1038/s41467-018-06395-8" @default.
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