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- W2890391341 abstract "We have recently reported a polymechanophore system, polyladderene (PLDE), which dramatically transforms into polyacetylene (PA) upon mechanical stimulation. Herein, we optimized conditions to synthesize unprecedented block copolymers (BCPs) containing a force-responsive block by sequential ring-opening metathesis polymerization of different norbornenes and bromoladderene. Successful extension from PLDE to other blocks required careful timing and low temperatures to preserve the reactivity of the PLDE-appended catalyst. The PLDE-containing BCPs were sonochemically activated into visually soluble PA with a maximum absorption λ ≥ 600 nm and unique absorption patterns corresponding to noncontinuous activation of ladderene units. Access to polymechanophore BCPs paves the way for new stress-responsive materials with solution and solid state self-assembly behaviors and incorporation of polymechanophores into other materials." @default.
- W2890391341 created "2018-09-27" @default.
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- W2890391341 date "2018-09-19" @default.
- W2890391341 modified "2023-09-30" @default.
- W2890391341 title "Synthesis and Mechanochemical Activation of Ladderene–Norbornene Block Copolymers" @default.
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- W2890391341 doi "https://doi.org/10.1021/jacs.8b08908" @default.
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