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• W2890406937 abstract "A range of amines catalyse the oxidative addition (OA) of H2 to [(Me3Si)2CH]2Sn (1), forming [(Me3Si)2CH]2SnH2 (2). Experimental and computational studies point to 'frustrated Lewis pair' mechanisms in which 1 acts as a Lewis acid and involve unusual late transition states; this is supported by the observation of a kinetic isotope effect for Et3N. When DBU is used the energetics of H2 activation are altered, allowing an equilibrium between 1, 2 and adduct [1·DBU] to be established, thus demonstrating reversible oxidative addition/reductive elimination (RE) of H2 at a single main group centre." @default.
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• W2890406937 date "2018-01-01" @default.
• W2890406937 modified "2023-10-15" @default.
• W2890406937 title "Base-induced reversible H₂ addition to a single Sn(<scp>ii</scp>) centre" @default.
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• W2890406937 doi "https://doi.org/10.1039/c8sc03110j" @default.
• W2890406937 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/6289099" @default.
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