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- W2890445616 abstract "For classical discrete systems under constant composition, it has been considered that genuine thermodynamic variables such as free energy cannot be generally determined from information about a single or a few selected microscopic states. Despite this fact, we here show that Helmholtz free energy for any given composition for disordered states can be well characterized by information about a few (R+3, where R denotes number of components) specially selected microscopic states, whose structure can be known a priori without requiring any thermodynamic information. The present study is a non-trivial extension of our recently-developed theoretical approach for special microscopic states in canonical ensemble to semi-grand canonical ensemble, which additionally enables to characterize temperature dependence of other thermodynamic variables such as internal energy and entropy." @default.
- W2890445616 created "2018-09-27" @default.
- W2890445616 creator A5068444403 @default.
- W2890445616 creator A5090048793 @default.
- W2890445616 date "2018-09-03" @default.
- W2890445616 modified "2023-09-25" @default.
- W2890445616 title "Formulation of Genuine Thermodynamic Variables from Special Microscopic States" @default.
- W2890445616 doi "https://doi.org/10.48550/arxiv.1809.00526" @default.
- W2890445616 hasPublicationYear "2018" @default.
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