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- W2890599595 abstract "Solid-state photochromic compounds can be used in molecular switch and memory, smart window, and so forth. However, a new photochromic mechanism was rarely reported. Photochromic Schiff bases without ortho-hydroxyl groups (thioamide hydrazones) have been prepared, which are drastically different from the traditional photochromic Schiff bases (e.g., salicylal anils and pyrazolone thiosemicarbazones). Systematic experimental and theoretical studies of thioamide hydrazone confirm the crystal-to-crystal photochromism and thermo-enhanced photochromism. The original faint yellow form changes to yellow after UV irradiation and can further be bleached by visible light irradiation. Besides, the decolored form can automatically change to yellow in dark at room temperature or by heating. The structures of the three forms (the original form, the colored form, and the decolored form) show that the intramolecular torsion and vibration lead to the increase/decrease of the donor (nitrogen atom)–acceptor (sulfur atom) dis..." @default.
- W2890599595 created "2018-09-27" @default.
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- W2890599595 date "2018-09-09" @default.
- W2890599595 modified "2023-10-18" @default.
- W2890599595 title "Molecular Orbital Delocalization/Localization-Induced Crystal-to-Crystal Photochromism of Schiff Bases without ortho-Hydroxyl Groups" @default.
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- W2890599595 doi "https://doi.org/10.1021/acs.jpcc.8b07408" @default.
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