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- W2890767168 abstract "We study photoinduced charge generation in a model polymer/nonfullerene acceptor (NFA) organic photovoltaic (OPV) blend. Specifically, we focus on hole-transfer kinetics from the photoexcited NFA thiophene-thieno[3,2-b]thiophene-thiophene-3-(dicyanomethylidene)indan-1-one (4TIC) to the conjugated polymer donor poly[(4,4′-bis(2-butyloctoxycarbonyl-[2,2′-bithiophene]-5,5-diyl)-alt-(2,2′-bithiophene-5,5′-diyl)] (PDCBT) using ultrafast transient absorption spectroscopy by selectively exciting the 4TIC electron acceptor and monitoring the bleach of the PDCBT ground-state population. In the blend, the 4TIC excitons decay with an average lifetime of 7 ps, accompanied by a concomitant rise in the ground-state bleach of the polymer with a comparable average lifetime that is 60% complete by 8 ps and 95% complete by 100 ps, occurring roughly an order of magnitude slower than that in most previously reported polymer/NFA blends. Notably, the ground-state bleach of the polymer continues to grow, not reaching its maximu..." @default.
- W2890767168 created "2018-09-27" @default.
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- W2890767168 date "2018-09-12" @default.
- W2890767168 modified "2023-10-06" @default.
- W2890767168 title "Unexpectedly Slow Yet Efficient Picosecond to Nanosecond Photoinduced Hole-Transfer Occurs in a Polymer/Nonfullerene Acceptor Organic Photovoltaic Blend" @default.
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- W2890767168 doi "https://doi.org/10.1021/acsenergylett.8b01416" @default.
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