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- W2890917462 abstract "Using molecular dynamics simulation of a polymer glass model we investigate free-standing polymer films focusing on the in-plane shear modulus $mu$ and the corresponding shear-stress relaxation modulus $G(t)$ as functions of temperature $T$, film thickness $H$ (tuned by means of the lateral box size $L$) and sampling time $Delta t$. Various observables are seen to vary linearly with $1/H$ demonstrating thus the (to leading order) linear superposition of bulk and surface properties. In agreement with recent studies on three-dimensional polymer glass-formers, $mu$ and $G(t)$ are found to decrease continuously with $T$. A jump-singularity is not observed. Confirming the time-translational invariance of our systems, the $Delta t$-dependence of $mu$ is traced back to $G(t)$." @default.
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- W2890917462 date "2018-12-04" @default.
- W2890917462 modified "2023-09-25" @default.
- W2890917462 title "Shear-stress relaxation in free-standing polymer films" @default.
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- W2890917462 doi "https://doi.org/10.1103/physreve.98.062502" @default.
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