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• W2890928882 endingPage "23563" @default.
• W2890928882 startingPage "23554" @default.
• W2890928882 abstract "Hierarchical architectures can transform inferior substances into high-performance materials. Although this effect is prevalent among biominerals, few examples in chemistry match the complexity of such ordered materials. One exception is the formation of “biomorphs”, which consist of co-aligned, crystalline nanorods that assemble into smoothly curved microstructures. These lifelike sheets, helices, and urns form when CO2 reacts with aqueous solutions of alkaline earth metals and silicate. For the case of SrCO3–silica biomorphs, micrometer-scale sheets form at the solution–air interface and begin to move due to convection with speeds of 1–10 μm/s. Short-range interaction via capillary forces induces the formation of clusters and eventually a single, centimeter-scale aggregate. Within this pattern, biomorphs are arranged into simple chains with some branching points yielding fractal dimensions of 1.2–1.3. Importantly, crystallization continues within the aggregate and diminishes internal motion. We show that the resulting structures are qualitatively different from those formed from solitary units and often include very large sheets connected to several biomorph units. Both aggregation and collective growth extend the hierarchical order to the centimeter scale and constitute a novel aspect of the system’s crystallization dynamics." @default.
• W2890928882 created "2018-09-27" @default.
• W2890928882 creator A5014528961 @default.
• W2890928882 creator A5052625397 @default.
• W2890928882 date "2018-09-19" @default.
• W2890928882 modified "2023-09-25" @default.
• W2890928882 title "Particle Aggregation Modifies Crystallization: Extending the Hierarchical Order of a Polycrystalline Material to the Macroscale" @default.
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• W2890928882 doi "https://doi.org/10.1021/acs.jpcc.8b07212" @default.
• W2890928882 hasPublicationYear "2018" @default.
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