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- W2891007254 abstract "A highly regio- and diastereoselective method to access cis-2,6-disubstituted dihydropyridinones under mild conditions by an iridium-catalyzed allylic etherification is reported. cis-2,6-Disubstituted dihydropyridinones are important precursors for the de novo synthesis of the corresponding piperidine alkaloids and iminosugars. This strategy features a broad substrate scope, high yields, and excellent regio- and diastereoselectivities. A π-allyl-Ir intermediate is involved in the mechanism. The strong A1,3-strain from the tosyl group may also favor the formation of cis-products in this transformation." @default.
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- W2891007254 date "2018-09-20" @default.
- W2891007254 modified "2023-10-10" @default.
- W2891007254 title "Iridium-Catalyzed Highly Regioselective and Diastereoselective Allylic Etherification To Access <i>cis</i>-2,6-Disubstituted Dihydropyridinones" @default.
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- W2891007254 doi "https://doi.org/10.1021/acs.joc.8b01598" @default.
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