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• W2891215489 abstract "Constructing appropriate cocatalysts to modify semiconductors while maintaining tight interface for charge separation facilitation is important for improving photocatalytic hydrogen production. Thus, in this work, C,N-codoped Fe2P/Ni2P (CN/FeNiP) polyhedrons derived from NH2-MIL-101(Fe)/Ni(OH)2 were used as cocatalysts to modify graphitic carbon nitride (g-C3N4) for photocatalytic hydrogen production from water splitting under visible-light irradiation. The highest evolution rate observed over CN/FeNiP/g-C3N4 was 13.81 mmol g−1 h−1 under 1.0 mmol L−1 of Eosin Y (EY) sensitization (compared to 0.196 mmol g−1 h−1 without EY sensitization), which was about 10 and 5 times higher than that of g-C3N4 (1.33 mmol g−1 h−1) and CN/FeP/g-C3N4 (2.73 mmol g−1 h−1). The apparent quantum yield at 420 nm reached 45.8%. A detail analysis of the mechanism revealed that the improved photocatalytic activity can be ascribed to highly efficient spatial separation of photo-induced charges from the excited EY and g-C3N4 to CN/FeNiP with tight interface, staggered band energy between g-C3N4, CN/Fe2P and Ni2P as well as accelerated surface reaction by CN/FeNiP cocatalysts. This work demonstrates that MOF-derived hybrid hollow metal phosphide can be good substitutes for noble metal catalysts for photocatalytic hydrogen production." @default.
• W2891215489 created "2018-09-27" @default.
• W2891215489 creator A5044717371 @default.
• W2891215489 creator A5053883844 @default.
• W2891215489 creator A5055838753 @default.
• W2891215489 creator A5062168859 @default.
• W2891215489 date "2019-02-01" @default.
• W2891215489 modified "2023-10-15" @default.
• W2891215489 title "NH2-MIL-101(Fe)/Ni(OH)2-derived C,N-codoped Fe2P/Ni2P cocatalyst modified g-C3N4 for enhanced photocatalytic hydrogen evolution from water splitting" @default.
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• W2891215489 doi "https://doi.org/10.1016/j.apcatb.2018.09.035" @default.
• W2891215489 hasPublicationYear "2019" @default.
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