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- W2891242561 endingPage "6125" @default.
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- W2891242561 abstract "An efficient strategy for the asymmetric synthesis of Cα-tetrasubstituted proline derivatives from proline has been established. A nitrogen-fused bicyclic system was devised to control the stereodynamics of proline. Through N-quaternizations with allylic electrophiles followed by [2,3]-rearrangements, the bicyclic proline system delivered enantioenriched Cα-tetrasubstituted prolines. This strategy was applied to the concise total synthesis of (-)-amathaspiramide F." @default.
- W2891242561 created "2018-09-27" @default.
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- W2891242561 date "2018-09-20" @default.
- W2891242561 modified "2023-10-16" @default.
- W2891242561 title "Asymmetric Cα-Alkylation of Proline via Chirality Transfers of Conformationally Restricted Proline Derivative: Application to the Total Synthesis of (−)-Amathaspiramide F" @default.
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- W2891242561 doi "https://doi.org/10.1021/acs.orglett.8b02568" @default.
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