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- W2891259659 endingPage "1803676" @default.
- W2891259659 startingPage "1803676" @default.
- W2891259659 abstract "Catalysts are at the heart of the hydrogen evolution reaction (HER) for the production of pure and clean hydrogen. For practical applications, the scalable synthesis of efficient HER catalysts, which work in both acidic and alkaline media, is highly desired. In this work, the mechanochemically assisted synthesis of a Ru catalyst with HER performance surpassing Pt in both acidic and alkaline media is reported. Mass production of this Ru catalyst can be achieved via a two-step procedure: the mechanochemical reaction between graphite and dry ice produces edge-carboxylic-acid-functionalized graphene nanoplatelets (CGnP); mixing a Ru precursor and the CGnP in an aqueous medium introduces Ru ions, which coordinate on the CGnP. Subsequent annealing results in uniform Ru nanoparticles (≈2 nm) anchored on the GnP matrix (Ru@GnP). The efficient Ru@GnP catalyst can be easily powered by a single silicon solar cell using a wireless integration device. The self-powered device exhibits robust hydrogen evolution under the irradiation of standard AM 1.5 solar light. This work provides a new opportunity for the low-cost mass production of efficient and stable catalysts for practical applications." @default.
- W2891259659 created "2018-09-27" @default.
- W2891259659 creator A5006894527 @default.
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- W2891259659 date "2018-09-14" @default.
- W2891259659 modified "2023-09-30" @default.
- W2891259659 title "Mechanochemically Assisted Synthesis of a Ru Catalyst for Hydrogen Evolution with Performance Superior to Pt in Both Acidic and Alkaline Media" @default.
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- W2891259659 doi "https://doi.org/10.1002/adma.201803676" @default.
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