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- W2891330516 abstract "The binding mechanism of Sb(V) on a single-crystal hematite (11̅02) surface was studied using crystal truncation rod X-ray diffraction (CTR) under in situ conditions. The best-fit CTR model indicates Sb(V) adsorbs at the surface as an inner-sphere complex forming a tridentate binding geometry with the nearest Sb-Fe distance of 3.09(4) Å and an average Sb-O bond length of 2.08(5) Å. In this binding geometry, Sb is bound at both edge-sharing and corner-sharing sites of the surface Fe-O octahedral units. The chemical plausibility of the proposed structure was further verified by bond valence analysis, which also deduced a protonation scheme for surface O groups. The stoichiometry of the surface reaction predicts the release of one OH- group at pH 5.5." @default.
- W2891330516 created "2018-09-27" @default.
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- W2891330516 date "2018-09-06" @default.
- W2891330516 modified "2023-10-14" @default.
- W2891330516 title "In Situ Structural Study of Sb(V) Adsorption on Hematite (11̅02) Using X-ray Surface Scattering" @default.
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- W2891330516 doi "https://doi.org/10.1021/acs.est.8b03903" @default.
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