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- W2891373731 abstract "Infrared pump-probe measurement for the OD stretching mode in KTaO3 has been performed. We observed the induced absorption signal corresponding to the 1-2 transition for the first time in oxide crystals in addition to the bleaching signal of the 0-1 transition. Both signals show long decay time of ∼200 ps, and the potential anharmonicity is found to be 3.6%. We also investigated temperature dependence of OH/OD absorption spectra to explore how a proton/deuteron interacts with the surrounding lattice vibrations, and identify the phonon mode which causes the potential fluctuations as a O–Ta–O bending motion. On the basis of the results obtained, we calculate the potential energy surface on which a proton/deuteron moves and discuss the proton conduction mechanism in solid oxides." @default.
- W2891373731 created "2018-09-27" @default.
- W2891373731 creator A5041377347 @default.
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- W2891373731 date "2018-09-12" @default.
- W2891373731 modified "2023-10-17" @default.
- W2891373731 title "Ultrafast proton/deuteron dynamics in KTaO3 observed with infrared pump-probe spectroscopy: Toward understanding of proton conduction mechanism in solid oxides" @default.
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- W2891373731 doi "https://doi.org/10.1063/1.5040063" @default.
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- W2891373731 hasPublicationYear "2018" @default.
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