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• W2891376110 abstract "Significance The understanding of a catalytic reaction starts with understanding its first elementary step. Surprisingly, despite the large number of studies, it is unclear whether one common or two different first intermediates control the selectivity of CO 2 electroreduction to formate and CO. We settle this controversy for Cu, which is best known for its unique capacity to synthesize C 1+ products but is just emerging as a superior earth-abundant catalyst for CO and formate. We provide solid experimental and theoretical support of the one common first-intermediate (Hori’s) model, the first intermediate being carboxylate. This outcome is an essential milestone toward accurate specification of the reaction descriptors in the growing effort to accelerate the discovery of a viable CO 2 electroreduction catalyst." @default.
• W2891376110 created "2018-09-27" @default.
• W2891376110 creator A5030519966 @default.
• W2891376110 creator A5031301453 @default.
• W2891376110 creator A5033600538 @default.
• W2891376110 date "2018-09-17" @default.
• W2891376110 modified "2023-10-14" @default.
• W2891376110 title "On the origin of the elusive first intermediate of CO ₂ electroreduction" @default.
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• W2891376110 doi "https://doi.org/10.1073/pnas.1802256115" @default.
• W2891376110 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/6176638" @default.
• W2891376110 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30224482" @default.
• W2891376110 hasPublicationYear "2018" @default.
• W2891376110 type Work @default.
• W2891376110 sameAs 2891376110 @default.

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