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• W2891378595 abstract "Triplet-excited-state-involved photonic and electronic properties have attracted tremendous attention for next-generation technologies. To populate triplet states, facile intersystem crossing (ISC) for efficient exciton spin-flipping is crucial, but it remains challenging in organic molecules free of heavy atoms. Here, a new strategy is proposed to enhance the ISC of purely organic optoelectronic molecules using heteroatom-mediated resonance structures capable of promoting spin-flipping at large singlet-triplet splitting energies with the aid of the fluctuation of the state energy and n-orbital component upon self-adaptive resonance variation. Combined experimental and theoretical investigations confirm the key contributions of the resonance variation to the profoundly promoted spin-flipping with ISC rate up to ≈107 s-1 in the rationally designed NPX (X = O or S) resonance molecules. Importantly, efficient organic ultralong room-temperature phosphorescence (OURTP) with simultaneously elongated lifetime and improved efficiency results overcoming the intrinsic competition between the OURTP lifetime and efficiency. With the spectacular resonance-activated OURTP molecules, time-resolved and color-coded quick response code devices with multiple information encryptions are realized, demonstrating the fundamental significance of this approach in boosting ISC dynamically for advanced optoelectronic applications." @default.
• W2891378595 created "2018-09-27" @default.
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• W2891378595 date "2018-09-10" @default.
• W2891378595 modified "2023-10-18" @default.
• W2891378595 title "Resonance-Activated Spin-Flipping for Efficient Organic Ultralong Room-Temperature Phosphorescence" @default.
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• W2891378595 doi "https://doi.org/10.1002/adma.201803856" @default.
• W2891378595 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30260515" @default.
• W2891378595 hasPublicationYear "2018" @default.
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