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• W2891396091 abstract "The first total syntheses of triptobenzene T, vitexifolin C, 4-epi-triptobenzene L, triptobenzene L, and nepetaefolin F have been accomplished through an enantioselective, common intermediate approach and have enabled the confirmation and/or establishment of the absolute stereochemistry of each natural product synthesized. Application of three new and/or underutilized Pummerer reaction pathways proved critical to the synthetic work. A proline sulfonamide-catalyzed Yamada–Otani reaction was used to access the highly functionalized cyclohexane A ring core, including the C10 all-carbon quaternary stereocenter. Additionally, the importance of the A ring unsaturation for controlling the stereoselectivity during the C4 alkylation is showcased." @default.
• W2891396091 created "2018-09-27" @default.
• W2891396091 creator A5022526821 @default.
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• W2891396091 date "2018-09-10" @default.
• W2891396091 modified "2023-10-18" @default.
• W2891396091 title "Total Syntheses of Aromatic Abietane Diterpenoids Utilizing Advances in the Pummerer Rearrangement" @default.
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• W2891396091 doi "https://doi.org/10.1021/acs.orglett.8b02060" @default.
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