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- W2891460030 endingPage "3964" @default.
- W2891460030 startingPage "3956" @default.
- W2891460030 abstract "Abstract The development of noble‐metal‐free, efficient, electrochemical, water‐splitting catalyst systems has attracted considerable attention in recent times. In this study, a metal–organic framework based synthetic route to couple two non‐noble‐metal‐based catalysts, CoP and Mo 2 C, supported on nitrogen‐doped carbon has been developed. The strategy enables the formation of a nanohybrid with an attractive pea‐like morphology, in which spherical CoP particles (≈10 nm) are embedded on two‐dimensional nitrogen‐doped carbon enriched with ultrafine Mo 2 C nanoparticles. This composition boosts the electrochemical alkaline water‐splitting reaction by showing overpotentials ( η 10 ) of only 94 and 265 mV for the hydrogen evolution reaction (HER) and oxygen evolution reaction (OER), respectively, at a current density of 10 mA cm −2 . Additionally, in an acidic medium, the η 10 values are 107 and 330 mV for HER and OER, respectively; this suggests good bifunctionality at both lower and higher pH levels. Overall water splitting has been demonstrated by the developed catalyst at a cell voltage of 1.64 V for a current density of 10 mA cm −2 in alkaline medium, and a constant current is produced for more than 40 h under chronoamperometric conditions. This study describes the combination of two nanocomponents, with interconnected surface structures, which result in highly active and stable electrocatalytic performance." @default.
- W2891460030 created "2018-09-27" @default.
- W2891460030 creator A5019059433 @default.
- W2891460030 creator A5034961161 @default.
- W2891460030 creator A5057149092 @default.
- W2891460030 creator A5073472607 @default.
- W2891460030 date "2018-10-24" @default.
- W2891460030 modified "2023-10-17" @default.
- W2891460030 title "An Intriguing Pea‐Like Nanostructure of Cobalt Phosphide on Molybdenum Carbide Incorporated Nitrogen‐Doped Carbon Nanosheets for Efficient Electrochemical Water Splitting" @default.
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- W2891460030 doi "https://doi.org/10.1002/cssc.201801810" @default.