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- W2891468729 abstract "Abstract The first total syntheses of asperchalasines A–E, a collection of unprecedented merocytochalasans, are reported. Aspochalasin B, a key tricyclic cytochalasan monomer, was first synthesized through a unified approach that hinges on a Diels–Alder reaction and a ring‐closing metathesis reaction. The bioinspired Diels–Alder reactions of aspochalasin B with different epicoccine precursors were then explored, which enabled the divergent access of the heterodimers asperchalasines B–E as well as related congeners. Furthermore, the heterotrimer asperchalasine A was obtained from one epicoccine unit and two aspochalasin B units through a biomimetic Diels–Alder reaction followed by an oxidative [5+2]‐cycloaddition." @default.
- W2891468729 created "2018-09-27" @default.
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- W2891468729 date "2018-10-04" @default.
- W2891468729 modified "2023-09-25" @default.
- W2891468729 title "Total Syntheses of Asperchalasines A-E" @default.
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- W2891468729 doi "https://doi.org/10.1002/anie.201808249" @default.
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