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- W2891472956 abstract "Abstract A lanthanide‐catalyzed intermolecular hydroamination of 2‐alkynylbenzonitriles with secondary amines has been disclosed, providing a streamlined access to a range of aminoisoindoles in moderate to excellent yields. The salient features of this reaction include high bond‐formation efficiency, mild reaction conditions, 100 % atomic efficiency and good functional group tolerance. This methodology has also been successfully applied to the construction of other nitrogen‐containing compounds, such as 5 H ‐imidazo[2,1‐ a ]isoindoles and isoquinolines. A plausible mechanism for the formation of aminoisoindoles involving initial N−H activation by a lanthanide complex followed by C≡N insertion into a Ln−N bond to form an amidinate lanthanide intermediate, which undergoes the cyclization is proposed." @default.
- W2891472956 created "2018-09-27" @default.
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- W2891472956 date "2018-11-08" @default.
- W2891472956 modified "2023-10-11" @default.
- W2891472956 title "Lanthanide‐Catalyzed Tandem Insertion of Secondary Amines with 2‐Alkynylbenzonitriles: Synthesis of Aminoisoindoles" @default.
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- W2891472956 doi "https://doi.org/10.1002/asia.201801252" @default.
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