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- W2891473820 abstract "Step-growth polymerization via C–H activation is an attractive technique due to its advantages such as atom- and step-economy, derived from the reduced the number of synthetic steps required for the overall process and elimination of organometallic byproducts. To expand the utility of C–H activation polymerization beyond C–C bond coupling, we recently developed a highly efficient direct C–H amidation polymerization (DCAP) involving C–N bond formation, as a green polymerization process for synthesizing polysulfonamides. Here, we present a full account of the use of DCAP in the preparation of a library of polysulfonamides and polyamide from various diamides and diazides. From extensive model studies, several directing groups were screened, and it was found that subtle design of the directing groups by altering the steric hindrance and chelating bond angle greatly affected the efficiency of C–H amidation. Five directing groups were selected and seven AA-type monomers and seven BB-type monomers of azides were..." @default.
- W2891473820 created "2018-09-27" @default.
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- W2891473820 date "2018-09-17" @default.
- W2891473820 modified "2023-09-24" @default.
- W2891473820 title "Library of Fluorescent Polysulfonamides and Polyamide Synthesized by Iridium-Catalyzed Direct C–H Amidation Polymerization" @default.
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- W2891473820 doi "https://doi.org/10.1021/acs.macromol.8b01405" @default.
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