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- W2891500141 abstract "Acrylic acid (AA) and its ester, methyl acrylate (MA), were produced by a green one-step aldol condensation reaction of dimethoxymethane and methyl acetate. The reaction was conducted over ZSM-35 zeolites with different concentrations of Brönsted acid, which were prepared by the sodium ion-exchange process with H-form zeolite. The acidic property of HZSM-35 was studied in detail through infrared experiments. About 51% of all bridging OH groups were distributed in cages, while 23% and 26%, respectively, were distributed in 10- and 8-ring channels. The catalytic performance was enhanced by a high concentration of Brönsted acid, indicating that Brönsted acid is an active site for the aldol condensation reaction. The ZSM-35 zeolite possessing a concentration of Brönsted acid as high as 0.049 mmol/g demonstrated excellent performance with a MA+AA selectivity of up to 73%." @default.
- W2891500141 created "2018-09-27" @default.
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- W2891500141 date "2018-11-01" @default.
- W2891500141 modified "2023-10-16" @default.
- W2891500141 title "HZSM-35 zeolite catalyzed aldol condensation reaction to prepare acrylic acid and its ester: Effect of its acidic property" @default.
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- W2891500141 doi "https://doi.org/10.1016/s1872-2067(18)63145-6" @default.
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