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- W2891576473 abstract "Nucleophilic reactivity of deconjugated butyrolactams has been demonstrated for enantioselective Michael additions to α,β-unsaturated aldehydes and ketones. These reactions are catalyzed by diphenylprolinol silyl ether and trans-1,2-diaminocyclohexane-derived bifunctional primary aminothiourea, respectively, producing the Michael adducts with moderate diastereoselectivities and good to excellent enantioselectivities (up to 99:1 er). Unlike in the case of structurally related deconjugated butenolides where vinylogous addition is prevalent, an exclusive α-addition is observed for deconjugated butyrolactams." @default.
- W2891576473 created "2018-09-27" @default.
- W2891576473 creator A5000823484 @default.
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- W2891576473 date "2018-09-04" @default.
- W2891576473 modified "2023-09-26" @default.
- W2891576473 title "Catalytic Enantioselective C–C Bond-Forming Reactions of Deconjugated Butyrolactams: Michael Addition to α,β-Unsaturated Aldehydes and Ketones" @default.
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- W2891576473 doi "https://doi.org/10.1021/acs.joc.8b02051" @default.
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