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- W2891605669 abstract "Abstract High-temperature sodium–sulfur batteries operating at 300–350 °C have been commercially applied for large-scale energy storage and conversion. However, the safety concerns greatly inhibit their widespread adoption. Herein, we report a room-temperature sodium–sulfur battery with high electrochemical performances and enhanced safety by employing a “cocktail optimized” electrolyte system, containing propylene carbonate and fluoroethylene carbonate as co-solvents, highly concentrated sodium salt, and indium triiodide as an additive. As verified by first-principle calculation and experimental characterization, the fluoroethylene carbonate solvent and high salt concentration not only dramatically reduce the solubility of sodium polysulfides, but also construct a robust solid-electrolyte interface on the sodium anode upon cycling. Indium triiodide as redox mediator simultaneously increases the kinetic transformation of sodium sulfide on the cathode and forms a passivating indium layer on the anode to prevent it from polysulfide corrosion. The as-developed sodium–sulfur batteries deliver high capacity and long cycling stability." @default.
- W2891605669 created "2018-09-27" @default.
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- W2891605669 date "2018-09-24" @default.
- W2891605669 modified "2023-10-17" @default.
- W2891605669 title "A room-temperature sodium–sulfur battery with high capacity and stable cycling performance" @default.
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- W2891605669 doi "https://doi.org/10.1038/s41467-018-06443-3" @default.
- W2891605669 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/6155237" @default.
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