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- W2891709929 endingPage "14234" @default.
- W2891709929 startingPage "14230" @default.
- W2891709929 abstract "Facile synthesis of fluorinated benzofurans from polyfluorophenols has been accomplished by means of a sigmatropic dearomatization/defluorination strategy composed of three processes: (1) interrupted Pummerer reaction of ketene dithioacetal monoxides with polyfluorophenols followed by [3,3] sigmatropic rearrangement, (2) Zn-mediated smooth reductive removal of fluoride from the dearomatized intermediate, and (3) acid-promoted cyclization/aromatization. Mechanistic investigations revealed important characteristic reactivity of polyfluorophenols in the present system. Some of the fluorinated benzofuran products were transformed by utilizing the 2-methylsulfanyl moieties." @default.
- W2891709929 created "2018-09-27" @default.
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- W2891709929 creator A5071931568 @default.
- W2891709929 creator A5074437907 @default.
- W2891709929 date "2018-10-02" @default.
- W2891709929 modified "2023-10-16" @default.
- W2891709929 title "Sigmatropic Dearomatization/Defluorination Strategy for C−F Transformation: Synthesis of Fluorinated Benzofurans from Polyfluorophenols" @default.
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- W2891709929 doi "https://doi.org/10.1002/anie.201809035" @default.
- W2891709929 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30211456" @default.
- W2891709929 hasPublicationYear "2018" @default.
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