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- W2891814825 abstract "The reaction between the 2,6‐di(pyrazol‐1‐yl)‐4‐(bromomethyl)pyridine ( L ) ligand and divalent transition metal salts led to the formation of three mononuclear complexes of formula [M( L ) 2 ](BF 4 ) 2 · x MeNO 2 [M = Fe II ( 1· x MeNO 2 ), x = 0 and 4, M = Co II , x = 2 ( 2·2MeNO 2 ) and]. Static magnetic measurements highlighted thermal spin crossover at high temperature (320–340 K) for the two Fe II solvatomorphs nevertheless both the solvation degree and crystal packing had drastic influence on the shape and width of the hysteresis loop. Thus the 1 displayed abrupt and straight (6 K) hysteresis loop while for 1·4MeNO 2 the thermal spin transition could be described as a six‐step gradual transition with the widest magnetic bistability range (35 K) for this kind of complexes. Irradiation at 530 nm of 1·4MeNO 2 provoked an efficient LIESST effect at low temperature (T LIESST = 55 K). Finally dynamic magnetic measurements of 2·2MeNO 2 shown a field‐induced mononuclear Single‐Molecule Magnet behavior with Δ = 14.6(4) cm –1 and τ 0 = 6.28(8) × 10 –7 s." @default.
- W2891814825 created "2018-09-27" @default.
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- W2891814825 date "2018-10-18" @default.
- W2891814825 modified "2023-10-16" @default.
- W2891814825 title "Spin‐Crossover and Field‐Induced Single‐Molecule Magnet Behaviour in Metal(II)‐Dipyrazolylpyridine Complexes" @default.
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- W2891814825 doi "https://doi.org/10.1002/ejic.201800819" @default.
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