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- W2891837172 abstract "Coordination bonds between catechol-functionalized proteins and metal ions serve as sacrificial bonds that play essential roles in the expression of good mechanical performance and the self-healing properties of mussel byssal threads, which has inspired researchers to develop a range of catechol-based functional polymers. Herein, we investigated the mechanical properties of catechol-functionalized network polymers crosslinked by dual coordination bonds, namely catechol-Ca and catechol-B. As the bonding strengths are different, the viscoelastic properties of these materials can be controlled by changing the relative concentrations of these two bonds. The dual-coordination polymer with a 75:25 ratio of catechol-B:catechol-Ca (PB75Ca25) exhibited a higher Young's modulus and break strength than the corresponding single-coordination polymer (PCa100 or PB1000). The chemical structure of the polymer itself remained unchanged; hence this is a facile experimental system for solely investigating the effects of dynamic bonds on the mechanical properties of network polymers." @default.
- W2891837172 created "2018-09-27" @default.
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- W2891837172 date "2018-06-25" @default.
- W2891837172 modified "2023-10-16" @default.
- W2891837172 title "Tuning the Mechanical Properties of Bioinspired Catechol Polymers by Incorporating Dual Coordination Bonds" @default.
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- W2891837172 doi "https://doi.org/10.2494/photopolymer.31.75" @default.
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