Matches in SemOpenAlex for { <https://semopenalex.org/work/W2891844212> ?p ?o ?g. }
- W2891844212 abstract "In many important cases, the rate of excitation of a system embedded in an environment is significantly smaller than the internal system relaxation rates. An important example is that of light-induced processes under natural conditions, in which the system is excited by weak, incoherent (e.g., solar) radiation. Simulating the dynamics on the time scale of the excitation source can thus be computationally intractable. Here we describe a method for obtaining the dynamics of quantum systems without directly solving the master equation. We present an algorithm for the numerical implementation of this method and, as an example, use it to reconstruct the internal conversion dynamics of pyrazine excited by sunlight. Significantly, this approach also allows us to assess the role of quantum coherence on biological time scales, which is a topic of ongoing interest." @default.
- W2891844212 created "2018-09-27" @default.
- W2891844212 creator A5003009913 @default.
- W2891844212 creator A5061216131 @default.
- W2891844212 date "2018-09-18" @default.
- W2891844212 modified "2023-10-16" @default.
- W2891844212 title "An efficient approach to the quantum dynamics and rates of processes induced by natural incoherent light" @default.
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- W2891844212 doi "https://doi.org/10.1063/1.5041005" @default.
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