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- W2891850878 abstract "The presence of mixed adsorption layers affects the mechanism and kinetics of irreversible Bi(III) ions electroreduction process in 2 mol·dm−3 chlorates(VII). Triton X-100 and Tween 80 change the dynamics of the catalytic activity of 6-mercaptopurine (6MP) on Bi(III) ions electroreduction with the tendency of inhibition. Above the critical micelle concentration of Triton X-100 and Tween 80, the irreversibility of Bi(III) ions electroreduction decrease to the size comparable to the irreversible reduction of Bi(III) in 2 mol·dm−3 chlorates(VII) which can be associated with the electrode surface blocking by formed hemispherical surface micelles. It was proved that the unstable complexes of Bi – 6MP or mixed Bi – 6MP – TritonX-100 and Bi – 6MP – Tween 80 intermediating in electrons transfer, play a significant role in the multi-stage mechanism of the electrode process. The hydration shell and composition of active complexes change as well. The obtained regularities indicate that in this case confirmed changes in entropy are a decisive factor." @default.
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- W2891850878 date "2018-11-01" @default.
- W2891850878 modified "2023-10-18" @default.
- W2891850878 title "The importance of the active complexes of 6 - mercaptopurine with Bi(III) with regards to kinetics and electrode mechanism changes in the presence of non-ionic surfactants" @default.
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- W2891850878 doi "https://doi.org/10.1016/j.jelechem.2018.09.026" @default.
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