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• W2891855320 endingPage "11630" @default.
• W2891855320 startingPage "11627" @default.
• W2891855320 abstract "We developed a highly regioselective addition of 1,3-dienes with simple ketones by nickel-hydride catalyst bearing DTBM-SegPhos ligand. A wide range of aromatic and aliphatic ketones directly coupled with 1,3-dienes, providing synthetically useful γ,δ-unsaturated ketones in high yield and regioselectivity. The asymmetric version of the reaction was also realized in high enantioselectivity by using novel chiral ligand DTBM-HO-BIPHEP. The utility of this hydroalkylation was demonstrated by facile product modification and enantioselective synthesis of ( R)-flobufen." @default.
• W2891855320 created "2018-09-27" @default.
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• W2891855320 date "2018-09-05" @default.
• W2891855320 modified "2023-10-17" @default.
• W2891855320 title "Nickel(0)-Catalyzed Hydroalkylation of 1,3-Dienes with Simple Ketones" @default.
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• W2891855320 doi "https://doi.org/10.1021/jacs.8b09346" @default.
• W2891855320 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30183283" @default.
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