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- W2891868565 abstract "FeII spin-crossover (SCO) coordination polymers of the Hofmann type have become an archetypal class of responsive materials. Almost invariably, the construction of their architectures has been based on the use of monotopic and linear ditopic pyridine-like ligands. In the search for new Hofmann-type architectures with SCO properties, here we analyze the possibilities of bridging ligands with higher connectivity degree. More precisely, the synthesis and structure of {FeII(LN3)[MI(CN)2]2}·(Guest) (Guest = nitrobenzene, benzonitrile, o-dichlorobenzene; MI = Ag, Au) and {FeII(LN4)[Ag2(CN)3][Ag(CN)2]}·H2O are described, where LN3 and LN4 are the tritopic and tetratopic ligands 1,3,5-tris(pyridin-4-ylethynyl)benzene and 1,2,4,5-tetrakis(pyridin-4-ylethynyl)benzene. This new series of Hofmann clathrates displays thermo- and photoinduced SCO behaviors." @default.
- W2891868565 created "2018-09-27" @default.
- W2891868565 creator A5025406526 @default.
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- W2891868565 creator A5060059837 @default.
- W2891868565 creator A5062928892 @default.
- W2891868565 creator A5085240842 @default.
- W2891868565 date "2018-09-12" @default.
- W2891868565 modified "2023-10-14" @default.
- W2891868565 title "Switchable Spin-Crossover Hofmann-Type 3D Coordination Polymers Based on Tri- and Tetratopic Ligands" @default.
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- W2891868565 doi "https://doi.org/10.1021/acs.inorgchem.8b01842" @default.
- W2891868565 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30207715" @default.
- W2891868565 hasPublicationYear "2018" @default.
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