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- W2891966014 abstract "Recent advances in graphene liquid cells for in situ transmission electron microscopy (TEM) have opened many opportunities for the study of materials transformations and chemical reactions in liquids with high spatial resolution. However, the behavior of thin liquids encapsulated in a graphene liquid cell has not been fully understood. Here, we report real time TEM imaging of the nanoscale dynamic behavior of liquids in graphene nanocapillaries. Our observations reveal that the interfaces between liquid and gas bubble can fluctuate, leading to the generation of liquid nanodroplets near the interfaces. Liquid nanodroplets often show irregular shape with dynamic changes of their configuration under the electron beam. We consider that the dynamic motion of liquid-gas interfaces might be introduced by the electrostatic energy from transiently charged interfaces. We find that improving the wettability of graphene liquid cells by ultraviolet-ozone treatment can significantly modify the dynamic motion of the encapsulated liquids. Our study provides valuable information of the interactions between liquid and graphene under the electron beam, and it also offers key insights on the nanoscale fluid dynamics in confined spaces." @default.
- W2891966014 created "2018-09-27" @default.
- W2891966014 creator A5003883118 @default.
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- W2891966014 date "2019-01-01" @default.
- W2891966014 modified "2023-10-14" @default.
- W2891966014 title "Dynamic behavior of nanoscale liquids in graphene liquid cells revealed by in situ transmission electron microscopy" @default.
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- W2891966014 doi "https://doi.org/10.1016/j.micron.2018.09.009" @default.
- W2891966014 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30265880" @default.
- W2891966014 hasPublicationYear "2019" @default.
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