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- W2891978007 abstract "The electronic influence on the catalytic properties in the semihydrogenation of acetylene is addressed by applying unsupported intermetallic materials from the solid solution Ga1–xSnxPd2 (0 ≤ x ≤ 1). Due to the only marginal changes in the crystal structure, the whole series shows excellent selectivity to ethylene (∼85%) comparable with the binary GaPd2. Moreover, the incremental addition of up to one electron per formula unit reveals a maximum in the specific catalytic activity around the nominal composition with x = 0.28 corresponding to 4.0 atom % tin in the near-surface region, as revealed by operando X-ray photoelectron spectroscopy measurements. The study shows a reliable and quantitative relation between the d-band shift and catalytic activity, revealing once more the potential of intermetallic compounds in heterogeneous catalysis." @default.
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- W2891978007 date "2018-09-03" @default.
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- W2891978007 title "Revealing Electronic Influences in the Semihydrogenation of Acetylene" @default.
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- W2891978007 doi "https://doi.org/10.1021/acs.jpcc.8b05732" @default.
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