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- W2892006019 abstract "Abstract The present work aims to investigate the effects of a CO 2 -rich atmosphere on the characteristics of coal-derived soot. The rapid pyrolysis of Shenfu bituminous coal was conducted in a Drop tube furnace (DTF) in N 2 and CO 2 atmospheres with a wall temperature of 1073–1473 K and residence time below 700 ms. The yields and microstructure characteristics of N 2 -soot and CO 2 -soot were analysed by using a series of techniques (elemental analysis, HRTEM, Raman, XRD, FT-IR and thermogravimetry techniques). CO 2 enhanced the soot formation and proceeded the dehydrogenation. CO 2 improved the order of internal carbon lattices, enhanced the lateral extension of carbon nanostructures, decreased the interplanar spacing of the graphene layers and also promoted the stack of polyaromatic layers. The variations of the SOLO, DUO, TRIO and QUARTO structures were also analysed, and the contribution of CO 2 was found to reduce the defects of the basic structure units (BSU). The defects of soot were an important indication of the initial gasification reactivity. Overall, CO 2 -soot was more mature and low active than N 2 -soot." @default.
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- W2892006019 date "2018-11-01" @default.
- W2892006019 modified "2023-10-17" @default.
- W2892006019 title "Effect of CO2 on the characteristics of soot derived from coal rapid pyrolysis" @default.
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- W2892006019 doi "https://doi.org/10.1016/j.combustflame.2018.05.033" @default.
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